He has favoured a 4-2-3-1 formation in the main, with Modric in the number 10 role.
Although playing further forward than he does for Real Madrid means Modric is involved less in the build-up than he is for his club, his influence is still huge - witnessed by his goal-scoring performance in the 3-0 win over Argentina in the group stages.
Modric touched the ball 62 times and made only 42 passes in that match but in the quarter-final win against Russia he was deployed further back, and had 139 touches and made 102 passes.
That did however mean Rakitic was a less influential figure, but if the two dovetail on Wednesday, England are likely to be starved of the ball.
Underdog status but first-class pedigree
In addition to Modric and Rakitic, there is high-level experience throughout Croatia's team, with many of the players at Europe's elite clubs, including Liverpool, AC Milan, Juventus, Atletico Madrid and Monaco.
They have won nine Champions Leagues between them, compared to England's one, and 11 of the 23-man squad have 40 caps or more.
Most of this team have been together for a decade, with key players such as Modric, Rakitic and Mario Mandzukic all making their debuts within a couple of years of each other in 2006 and 2007.
"What I adore about them the most is their commitment to the national jersey," said Tomislav Dasovic of Vecernji List newspaper.
The feeling in Croatia is they are now at their peak as a team - and have never been happier as a group.
"They are good mates off the pitch, but most importantly they believe in the coach," added Dasovic. "He knows how to speak to them, he knows their DNA."
Resilient and driven by pain of 2016
Highlights: Croatia 1-1 Denmark (3-2 on pens)
While England left Euro 2016 embarrassed by Iceland, Croatia departed wondering what might have been.
They lost a tight last-16 tie against Portugal by conceding the only goal of the game at the end of extra time in a match in which they had the majority of possession and had 17 shots to their opponents' six.
Had they won, Poland and Wales would have stood between Croatia and a final against host nation France.
Their gutsy displays in this World Cup against Denmark and Russia - Modric missed a late penalty against the former and Croatia conceded a late equaliser against the latter but went on to win both games on penalties - speak of a side with a strong character which is determined to make the most of their opportunity this time.
Who will strike the latest blow?
Steve McClaren
McClaren was dubbed the "wally with the brolly" after England's failure to reach Euro 2008
This will be the eighth meeting between the two sides, with England winning four, Croatia twice and one draw.
They have only met in a major tournament once, at Euro 2004, when England's then teenage striker Wayne Rooney scored twice.
Croatia got their revenge during Euro 2008 qualifying as they won 3-2 at Wembley as England failed to reach the finals in a match remembered for boss Steve McClaren sheltering from the rain under an umbrella.
Two years later, Theo Walcott's only international hat-trick came against Croatia as England qualified for the 2010 World Cup.
In this World Cup, Croatia topped their group with a 100% winning record ahead of Argentina, but have scraped through knockout games against Denmark and the hosts via penalties.
"We have worked through difficult matches, some of them better than others," said Dalic.
"We respect England, we are a bit anxious because they are a great team. But England are not better than us! We respect them - they are a young and promising team. They are a very difficult opponent.
"We are happy with what we have achieved so far. We are among the four best teams in the world. We have nothing but respect for England, Belgium and France, but none of these teams is better than us."
All you need to know about Croatia
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